Something that a lot of muzzleloading shooters don't know is that if you shoot mainly patched balls, as I have for most of my life, then lead hardness is not as critical as it is when shooting lead conicals.
Depending upon the depth of the grooves, simply moving to a slightly smaller ball diameter may be the only change necessary to substantially increase the hardness of the lead used in casting the balls. This is true due to the ability of a thick patch to compress far more than most people believe is possible.
One needs to be utilizing patches that measure, compressed under the jaws of a micrometer/vernier caliper, at least 0.020" thick, or thicker, for the above statement to be applicable.
Increased lead hardness, over a pure lead ball, usually results in a ball that drops from the mold measuring slightly larger in diameter than one cast from pure lead.
If one desires to cast balls, for example, from pure wheel weight metal, or linotype metal, both of which measure quite hard on the Brinnel scale, then it may be necessary to reduce the diameter of the cast balls by as much as 0.015" in order to maintain the same accuracy as with a pure lead ball.
All barrels are unique, and what works for one barrel, may require a completely different ball diameter, and or patch thickness, in order to obtain the same standards of accuracy. This is true, even with barrels from the same manufacturer that to all appearances measure out as identical.